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Ultrathin 2D metal nanostructures have sparked a lot of research interest because of their improved electrocatalytic properties for fuel cells. So far, no effective technique for preparing ultrathin 2D Pd‐based metal nanostructures with more than three compositions has been published. Herein, a new visible‐light‐induced template technique for producing PdAuBiTe alloyed 2D ultrathin nanosheets is developed...