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Quasi‐amorphous thin films of BaTiO3, SrTiO3, and BaZrO3 are the only known examples of inorganic, non‐crystalline, polar materials. The conditions under which they are formed and the origin of their polarity set these materials apart from other classes of inorganic materials. The most important feature of the quasi‐amorphous phase is that the polarity is the result of the orientational ordering of...
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