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In article number 1802169, Jiaguo Yu, Hao Ming Chen, and co‐workers demonstrate the construction of a single‐atom engineered Pd/g‐CN hybrid with directional charge transfer channels and targeting active sites by interlayer intercalation and a surface anchor of Pd atoms. This unique material shows excellent charge transfer/separation and efficient photocatalytic hydrogen evolution.
Efficiency of layered photocatalysts such as graphitic carbon nitride (g‐CN) is still too low due to the poor utilization of photoexcited‐charge carriers. The major drawback is that the weak van der Waals force among g‐CN layers is unfavorable for the charge transfer between the adjacent layers and the intrinsically π‐conjugated planes with inefficient random in‐plane charge migration. Herein, an...
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