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Manganese hexacyanomanganates have attracted significant attention as promising cathode materials for sodium‐ion batteries owing to the high theoretical capacity and low cost of Mn resources. Because of the strong Jahn–Teller effect, causing unstable local phase transition and distortion, the redox reactions of the high‐spin state of Mn(III) are considered to be a conundrum. Herein, it is reported...
Charge Redistribution
In article number 2111901, Young Hwa Jung, Hyun‐Wook Lee, and co‐workers demonstrate that the fast reaction rate activates charge redistribution in manganese hexacyanomanganates, which can mitigate the strong Jahn–Teller effect of high‐spin Mn(III) by solving the unequal number of electrons in eg orbitals. As a result, the dissolution of Mn is effectively suppressed, inducing...
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