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In article number 2008712, Meysam Heydari Gharahcheshmeh, Karen K. Gleason, and co‐workers present remarkable texture and nanostructural engineering of poly(3,4‐ethylenedioxythiophene) (PEDOT) thin films grown by water‐assisted oxidative chemical vapor deposition, which yields a record high electrical conductivity of 7520 S/cm. In PEDOT thin films with a highly face‐on orientation, the charge transport...
Engineering the texture and nanostructure to improve the electrical conductivity of semicrystalline conjugated polymers must address the rate‐limiting step for charge carrier transport. In highly face‐on orientation, the charge transport between chains within a crystallite becomes rate‐limiting, which is highly sensitive to the π–π stacking distance and interchain charge transfer integral. Here, face‐on...
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