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Body‐centered cubic (BCC) and high‐entropy alloys are being investigated as potential hydrogen storage materials due to their ability to absorb high amounts of hydrogen at moderate temperatures. Herein, the synthesis and hydrogen storage behavior of new MgVCr BCC and MgTiVCrFe high‐entropy alloys are studied. The alloys are initially synthesized by mechanical alloying via high‐energy ball milling...