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In some real and up-scale tests using high-level radioactive waste (HLRW), Mg accumulation was observed in smectites at the contact of heated Fe or Cu metal tubes. It is important to understand why Mg accumulated in order to model the long term performance of bentonites in HLRW systems. In some of these tests, an increased number of trioctahedral domains was measured in the smectites using X-ray diffraction...
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