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The confined crystallization behavior of polycaprolactone (PCL) in thin and ultrathin films was studied by AFM (atomic force microscopy). It was found that the crystalline morphology of PCL depended on the film’s thickness. When the thickness is d > 2 Rg (radius of gyration), the polymer can crystallize into spherulites; when Rg < d < 2 Rg, a dense-branch morphology and dendrites could be...
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