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The promotion effect of transition metal on the catalytic performance of a Pd catalyst for the direct synthesis of 3-picoline from 2-methylglutaronitrile was investigated. The PdZn/SiO2–Al2O3 catalysts with appropriate Zn/Pd molar ratio exhibited a high 3-picoline yield. Kinetic and mechanism analysis revealed a kinetically relevant step of dehydrogenation in 3-methyltetrahydropyridine to 3-picoline...
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