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N-(Acetylamino)phthalimide [monoclinic, a = 7.0228(15), b = 4.7285(8), c = 28.882(6) Å, β = 90.131(7)°, space group P21/c] shows an unusual crystal structure with marked pyramidalization at the phthalimide N and strong intermolecular NH to CO hydrogen bonding leading to the groups at the two ends of the hydrazine adopting an almost perpendicular arrangement. A survey of previous triacyl and tetraacyl...
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