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With the catalysis of K2PdCl4 and H5PMo10V2O40 in CF3COOH, methane can be oxidized into CH3COOH and CF3COOCH3 using molecular oxygen as the oxidant at a low temperature. H5PMo10V2O40 is a reversible oxidant that allows to retain Pd(II) in CF3COOH and thus to complete a two-step catalytic cycle of oxidation of methane by molecular oxygen; in addition, it can catalytically oxidize methane into CH3COOH...
A water-tolerant, active and high-selective palladium catalyst, (2,2′-bipyridine) dichloropalladium(II) is proposed for the oxidation of methane to a methanol derivative with molecular oxygen as the oxidant at temperatures below 120 °C, and its activity can be increased by three times at 100 °C when the volume ratio of water to CF3COOH solvent is 1:5. In addition, the addition of perfluorooctane can...
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