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XPS and Δφ measurements demonstrate that the potential of a Rh thin film in contact with a Na + conducting solid electrolyte may be used to control ϑ Na and hence the catalytic behaviour of the Rh surface. The system response is reversible and reproducible, catalyst work function and Na coverage varying linearly with catalyst potential over the experimentally accessible range. Coordinated...
Adsorption and co-adsorption of nitric oxide (NO) and carbon monoxide (CO) on a Pd(111) surface were studied using pseudopotential density-functional theory calculations. For individual NO and CO molecules we determined the energetically most stable adsorption sites and harmonic frequencies. The results show that at 0.25 monolayer (ML) coverage both the molecules prefer to reside on a hollow site...
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