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Monolayer films of Co on Cu(001) annealed at 180 o C exhibit ordered c(2x2) regions as evidenced by STM images. The ordered surface alloy formation of Co-Cu(001) in the monolayer regime occurs in spite of the bulk immiscibility of Co-Cu and in contrast to the theoretically predicted instability of a c(2x2) ordered monolayer. RHEED and LEED exhibit superstructure-related reflections that corroborate...
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