The molecular beam epitaxy growth techniques which have already successfully produced a range of heavy rare-earth superlattices have now been extended to produce superlattices of two light rare-earth elements, Nd/Pr, as well as superlattices and alloy films of a heavy/light system, Ho/Pr. High-resolution X-ray diffraction analysis shows the Nd/Pr superlattices to be of high structural quality, while the Ho/Pr superlattices are significantly less so. In the Ho/Pr superlattices, Pr is found to retain its bulk dhcp crystal structure even in thin layers (down to 6 atomic planes thick) sandwiched between thick layers of hcp Ho. In addition, neutron diffraction studies of the Ho/Pr superlattices have shown that the helical Ho magnetic order is not coherent through the dhcp Pr layers, in contrast to previous hcp/hcp superlattices Ho/Y, Ho/Lu and Ho/Er. The series of Ho:Pr alloy films has shown structural trends similar to bulk alloys, with a range of compositions between Ho 0 . 5 5 Pr 0 . 4 5 and Ho 0 . 3 5 Pr 0 . 6 5 where the Sm δ-structure is stable, separating more extensive regions of hcp and dhcp solid solutions.