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An Al2O3-doped Li6.4La3Zr1.4Ta0.6O12 (LLZTO) cylinder with a cubic garnet structure was prepared by solid state reaction and pressureless sintering. The LLZTO cylinder showed a high relative density of ~94%. LLZTO sheets (200μm in thickness) were obtained by slicing the LLZTO cylinder using a low speed diamond saw. Ionic conductivity of the sheet was as high as 1.02×10−3S·cm−1 at room temperature...
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