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In the search of new probes for in vivo brain imaging of vesicular monoamine transporter type 2 (VMAT2), we have developed an efficient synthesis of a novel series of 3-alkyl-dihydrotetrabenazine (DTBZ) derivatives. The affinity of VMAT2 was evaluated by an in vitro inhibitory binding assay using [ 125 I]-iodovinyl-TBZ or [ 18 F](+)-FP-DTBZ as radioligands in rat striatal tissue homogenates...
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