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We present an atomic-scale investigation of the molecular interactions relevant to hydrodesulfurization (HDS) catalysis at the catalytically active edge sites of single-layer MoS2 and cobalt-promoted MoS2 (CoMoS) nanoparticles synthesized as model catalysts. Atom-resolved scanning tunneling microscopy observations of the adsorption of thiophene, pyridine, and various refractory alkyl-substituted dibenzothiophenes...
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