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Herein we report H-AlMCM-41 aluminosilica supported Ir materials with adjusted acid/metal function as bifunctional catalysts for selective ring opening (RO) of 1,2-dimethylcyclohexane (1,2-DMCH) at 330°C and 3MPa to primary ring opening products (P-ROP), which are defined as C8 alkanes. Large-pore H-AlMCM-41 materials were synthesized with Si/Al atomic ratios of 20 and 45 and impregnated for the first...
This study considers the thermochemistry and kinetics of γ-valerolactone and pentenoic acid interconversion as well as the decarboxylation of both molecules over amorphous silica alumina. Through microkinetic analysis, macroscopically observed production rates and product distributions are reconciled with a mechanistic description of all chemistries. Ring opening of γ-valerolactone, cyclization of...
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