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The manganese clusters have attracted much attention in relation with the oxygen evolving center (OEC) in photosystem II (PS II) system, which catalyzes the water oxidation reaction. Previously, we examined various spin-structures of Mn(II) 4 O 4 model clusters, of which all of magnetic interactions are antiferromagnetic. In this study, we investigated electronic and magnetic structures...
A new mixed-valence [Mn 9 ] cluster of formulae [Mn 9 O(OH) 3 Cl 4 (N 3 ) 3 (hmp) 6 (dpkd) 3 ]·1.5CH 3 CN·3H 2 O (1·1.5CH 3 CN·3H 2 O, where hmp − and dpkd 2− are the anion of 2-hydroxymethylpyridine and the dianion of the gem-diol form of the dpk, respectively) has been synthesized and...
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