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The addition of nucleophiles X - (X = H, D, OH, CN) to the complex cation [Ru(η 6 -C 6 H 6 )(Pz 3 BH)] + proceeds smoothly to give the neutral cyclohexadienyl compounds [Ru(η 5 -C 6 H 6 X)(Pz 3 BH)] which are identified by NMR spectroscopy and single crystal X-ray diffraction (for X = CN).