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By combining structural, morphological, spectroscopic and electrochemical information on the kinetics of epitaxial Pt thin film electrodes we obtain a detailed picture of the Pt/YSZ electrode. A route to tailor-made model type electrodes is discussed.
Thin Platinum films, prepared by Pulsed Laser Deposition (PLD) on single-crystalline yttria-stabilized zirconia (YSZ), show microstructurally uncontrolled dewetting upon heating to elevated temperatures. We tested several methods to induce the dewetting process, yielding a regular pattern — including structuring by masking of the surface with a Pt net and pre-coating of the YSZ surface with different...
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