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This study is focused on the influence of impurities and electrode morphology on cyclic voltammograms (CV) of one of the most prominent solid state electrode systems, Pt(O 2 )|YSZ, exemplifying the difficulties in unequivocal interpretation of CV in the solid state in general. By investigating differently prepared electrodes—either by Pt paste or pulsed laser deposition (PLD)—with and without...
The effect of sodium-modification on the catalyst and electrocatalytic properties of a platinum catalyst supported on a YSZ solid electrolyte was studied. Increasing the sodium coverage on the catalyst surface appears to block some of the three-phase boundary (tpb) sites and reduces the rate of the charge transfer reaction. The promotion of the platinum surface reaction (ethylene oxidation) seems...
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