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Using dynamic, mass budget, and empirical models, we quantified sulphate–sulphur (SO 4 –S) leaching from soils in a large central European catchment (upper Vltava river, Czech Republic) over a 110-year period (1900–2010). SO 4 –S inputs to soils with synthetic fertilisers and atmospheric deposition increased in the 1950s–1980s, then rapidly decreased (~80%), and remained low since...
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