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Second order nonlinear optical properties of the Zn-doped lithium niobate single crystals have been quantitatively studied from the chemical bond viewpoint. The results show that the second order nonlinear optical response of Zn-doped LiNbO 3 single crystals at 1079 nm decreases linearly with increasing Zn concentration in the crystal. This linear correlation is quantitatively expressed in...
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