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An electron-accepting building block, thieno[3,4-d]thiazole (TTz) was synthesized through a new synthetic route. When it was alternatively copolymerized with electron-donating fluorene, carbazole, or benzodithiophene derivatives via coupling reaction, all of the three copolymers had the low-lying lowest occupied molecular orbital energy levels around −3.55eV, while the highest occupied molecular orbital...
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