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The mechanism of the magnetic coupling in the [CuMCu(pda) 4 Cl 2 ] complexes with M=Pd, Pt is analyzed. First principles calculations based on the wave function theory are performed (DDCI+SO-RASSI): it is shown that the interaction without spin-orbit coupling is antiferromagnetic while the contribution due to the spin-orbit is ferromagnetic. The agreement between calculations and experiment...
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