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The direct tert-butyl group transfer was observed between t-BuBNAH and (η 6 -arene)Mn(CO) 3+ complexes in reflux acetonitrile without a radical initiator, and the corresponding tert-butyl radical addition products were achieved. The substituents on the aromatic ring significantly influence the reactivity and chemoselectivity. The electron-withdrawing group helps to promote the...
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