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A bottom‐up approach is introduced to fabricate two‐dimensional self‐assembled layers of molecular spin‐systems containing Mn and Fe ions arranged in a chessboard lattice. We demonstrate that the Mn and Fe spin states can be reversibly operated by their selective response to coordination/decoordination of volatile ligands like ammonia (NH3).
Addressable arrangements of spins at the molecular scale provide novel and exciting possibilities towards future spintronic applications. On page 2404, Nirmalya Ballav, Christian Wäckerlin, and co‐workers employ a bottom‐up approach to build a two‐dimensional array containing paramagnetic Mn and Fe complexes arranged in a chessboard‐like lattice. On‐surface magnetochemistry allows for the selective...
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