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Spatially resolved species and temperature profiles measured for a wide range of inlet stoichiometries and flowrates are compared with microkinetic numerical simulations to investigate the effect of transport phenomena on the catalytic partial oxidation of methane on Rh foam catalysts. In agreement with the experimental data, the species profiles calculated at different C/O inlet stoichiometries show...
Using spatially resolved measurements of temperature and concentration, we critically analyzed the chemistry and transport limitations in the partial oxidation of methane (POM) reaction carried out on Rh, supported on a foam catalyst. The analysis was based on two models, both sharing a detailed surface chemistry but with different gas–surface transport processes. The simulation neglecting transport...
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