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The reactivity of ZnMe2 towards heteroleptic (poly)hydride ruthenium complexes was investigated. The Ru centers were coligated with different ligands including reactive low‐valent ECp* (E = Ga, Al; Cp* = pentamethylcyclopentadienyl) ligands and nonreactive phosphane ligands (PCy3, PPh3, Cy = cyclohexyl, Ph = phenyl). The ECp* ligands undergo a redox reaction together with Cp*/Me group exchange when...
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