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Composition effect on electro-optic (EO) properties of a LiNbO₃ (LN) single-crystal has been investigated in a Li₂O-content range of 47.0-49.95 mol%. Some non-congruent LN crystals with different Li₂O-contents were prepared by performing Li-deficient or Li-rich vapour transport equilibration treatments on as-grown congruent LN crystals. Unclamped EO coefficients γ₁₃ and γ₃₃ of these samples were measured...
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