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The challenge with aqueous zinc‐ion batteries (ZIBs) lies in finding suitable cathode materials that can provide high capacity and fast kinetics. Herein, two‐dimensional topological Bi2Se3 with acceptable Bi‐vacancies for ZIBs cathode (Cu‐Bi2−xSe3) is constructed through one‐step hydrothermal process accompanied by Cu heteroatom introduction. The cation‐deficient Cu‐Bi2−xSe3 nanosheets (≈4 nm) bring...
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