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Single‐ion magnets (SIMs) are the smallest possible magnetic devices and are a controllable, bottom‐up approach to nanoscale magnetism with potential applications in quantum computing and high‐density information storage. In this work, we take advantage of the promising, but yet insufficiently explored, solid‐state chemistry of metal–organic frameworks (MOFs) to report the single‐crystal to single‐crystal...
Solid‐state incorporation of a single‐ion magnet (SIM) within the pores of a magnetic 3D metal–organic framework (MOF) in a single‐crystal to single‐crystal process has been demonstrated. The resulting host–guest supramolecular aggregate affords the first deep study on the interplay of the internal magnetic field of the MOF and the slow magnetic relaxation of the SIM allowing the observation of a...
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