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Liquid organic hydrogen carriers (LOHCs) have great potential as a hydrogen storage medium needed for a future sustainable energy system. Dehydrogenation of LOHCs requires a catalyst, such as supported Pd nanoparticles. Under reaction conditions, hydrogen and carbon may diffuse into the bulk of supported Pd catalyst particles and affect their activity and selectivity. The detailed understanding of...
Combining molecular beam (MB) techniques, reflection–absorption infrared spectroscopy (RAIRS), and temperature-programmed desorption (TPD), we have investigated the adsorption and kinetics of conversion of cis- and trans-2-butene with deuterium on a well-defined model supported Pd catalyst. Particular emphasis was placed on the quantitative comparison of the reaction rates of the competing cis-trans...
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