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The role that LiBr plays in the lifetime of Pd‐NHC complexes has been investigated. A bromide ion is proposed to coordinate to Pd thereby preventing beta hydride elimination (BHE) (to form NHC‐H+) of the reductive elimination (RE) intermediate that normally completes with the desired cross‐coupling catalytic cycle. Coordinating groups, such as anilines, are able to bind suitably well to Pd to prevent...
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