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While many operando techniques focus on gas phase reactions, there is a growing need to look at working catalysts in the liquid phase. Fluorescence microscopy is a promising technique for bridging this phase gap. Like cellular biology, catalytic science may take advantage from the high spatiotemporal resolution and sensitivity of fluorescence microscopy. Earlier applications of fluorescence techniques...
Careful combination of a metal compound,a ligand and an inorganic support material leads to supramolecular catalysts that mimic the structural, organizational and functional aspects of enzyme activity.After discussing essential features of metalloenzyme-catalyzed reactions and coordination chemistry in inorganic hosts, we present examples of supramolecular materials selected from our own work that...
Mg,Al-Layered double hydroxides (LDHs) are pillared with vanadium under mildly acidic conditions. Via XRD, Raman, and IR characterization, it is confirmed that the material is a phase-pure LDH with decavanadate (V 10 O 286− ) anions between the brucite sheets. This V 10 -LDH has the highest activity for the epoxidation of geraniol when used with tert-butyl hydroperoxide...
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