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With revealing the evolution of the B–O–B bond angle, Shouhua Feng and co‐workers demonstrate in article number 1803513 the structure–effect relationship between B–O bond covalency and oxygen reduction reaction performance in ABO3‐type perovskite oxides. This work is devoted to offering a fundamental theoretical and technical insight into precise regulation of electronic structure through design and...
Identifying the relationship between catalytic performance and material structure is crucial to establish the design principle for highly active catalysts. Deficiency in BO bond covalency induced by lattice distortion severely restricts the oxygen reduction reaction (ORR) performance for ABO3‐type perovskite oxides. Herein, a rearrangement of hybridization mode for BO bond is used to tune the overlap...
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