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Defective metal–organic frameworks are highlighted in article number 1704501 by Gregor Kieslich, Roland A. Fischer, and co‐workers. Besides synthesis and characterization, recent developments from computational aspects over functions toward potential applications of these materials are reviewed.
The targeted incorporation of defects into crystalline matter allows for the manipulation of many properties and has led to relevant discoveries for optimized and even novel technological applications of materials. It is therefore exciting to see that defects are now recognized to be similarly useful in tailoring properties of metal‐organic frameworks (MOFs). For instance, heterogeneous catalysis...
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