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Polymer‐based quasi‐solid‐state electrolyte (QSE) is an effective means to solve the safety problem of lithium (Li) metal batteries, and stable solid‐electrolyte‐interface (SEI) layers between electrolyte and anode/cathode are highly required for their long‐term stability. Herein, it is demonstrated that a silicon‐doped polyether functions as a multifunctional unit, which can induce the formation...
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