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The dealing/recycling of Ni‐containing wastewater pollution has aroused great attention both from environmental science and resource utilization perspectives. Herein, a classic CaFe‐layered double hydroxide (CaFe‐LDH) stabilizer, which exhibits a super‐stable mineralization efficiency for removing Ni2+ ions with a maximum saturated removal capacity of 321 mg g−1 is prepared. This stabilizer can remove...