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A small‐scale standalone device of nitrogen (N2) splitting holds great promise for producing ammonia (NH3) in a decentralized manner as the compensation or replacement of centralized Haber–Bosch process. However, the design of such a device has been impeded by sluggish kinetics of its half reactions, i.e., cathodic N2 reduction reaction (NRR) and anodic oxygen evolution reaction (OER). Here, it is...
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