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The valence excitation spectra of the copper tetrachloride and copper tetrabromide open-shell dianions, CuCl42- and CuBr42-, respectively, are investigated by a variety of symmetry-adapted-cluster configuration-interaction (SAC-CI) and equation-of-motion coupled-cluster (EOMCC) methods. The valence excited states of the CuCl42- and CuBr42- species that correspond to transitions from doubly occupied...
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