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Dynamics and inertia: The rotation of the CF3 top in α,α,α‐trifluorotoluene becomes considerably hindered by a V3 barrier in α,α,α‐trifluoro‐p‐tolualdehyde. Situated in a local V6 environment, the V3 barrier is caused by the aldehyde group and communicated through the aromatic π system. Quite dramatically, the ground state inertial defect jumps from −1.271 to −89.961 uÅ2, thus reflecting the electronically...
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