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N‐annulated perylenedicarboxamides 1–3 form supramolecular polymers with a strong tendency to aggregate. The bundles of fibers formed generate a spontaneous anisotropy that conditions the chiroptical features of the described molecules in solution; a strong linear dichroism effect accompanies the circular dichroism (CD) outcome. There is no influence of the point chirality existing at the side chains...
Chirality constitutes a source of inspiration for scientists. The oscillating helicity detected for the supramolecular polymers formed by the self‐assembly of three N‐annulated perylenedicarboxamides is described in article number 1603880, by Enrique Ortí, and Luis Sánchez, and co‐workers. The cooperative supramolecular polymerization of these compounds generates helical, chiral supramolecular structures,...
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