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A series of transition‐metal organometallic complexes with commonly occurring metalchlorine bonding motifs were characterized using 35Cl solid‐state NMR (SSNMR) spectroscopy, 35Cl nuclear quadrupole resonance (NQR) spectroscopy, and first‐principles density functional theory (DFT) calculations of NMR interaction tensors. Static 35Cl ultra‐wideline NMR spectra were acquired in a piecewise manner at...
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