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Measurements are reported for sequential clustering of CH 4 to Co + ions under equilibrium conditions. The CH 4 cluster bond strengths show a pairwise behavior: −ΔH 00 = 23.1 and 25.3 kcal/mol for n = 1 and 2; 7.3 and 5.2 kcal/mol for n = 3 and 4; and ∼2 kcal/mol for both n = 5 and 6. This pairwise behavior is well reproduced by large basis set density functional...
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