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Poly(1,1-silole)s were synthesized for the first time in 1999, by us and by West and his coworkers, as a new type of polysilane which is expected to have a low-lying LUMO due to the σ*-π*conjugation characteristic of the silole ring. Summarized herein are the development of new synthetic methodologies and the structural aspects, photophysical properties and a unique reactivity of the resulting oligo-...
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