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The vibration–rotational spectrum of the Ar–N2O van der Waals complex has been recorded in the low-frequency stretching mode region of the N2O-monomer (ν1∼1285cm−1). Almost 400 absorption lines were detected using a free supersonic slit-jet expansion in combination with an infrared tunable diode laser spectrometer. The recorded spectrum was assigned to the ν2-band of Ar–N2O. Rotational constants as...
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