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A structural transition has been observed in a digital superlattice of La2/3Sr4/3MnO4, which is correlated to a magnetization enhancement upon cooling the sample. These artificial superlattices were grown layer‐by‐layer using ozone‐assisted molecular beam epitaxy (MBE). Electron diffraction experiments show a phase transition below 150 K in nanopatches of the superlattice, which coincides with an...
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