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A mixture of the building blocks 1A and 2G, featuring d‐alanine moieties and glycine‐functionalized calix[4]arene moieties, respectively, formed a co‐assembled hydrogel. In particular, the remarkable enhancement of helical intensity of co‐assembled gel was controlled by achiral calix[4]arene 2G, which was attributed to the bridging effect between 1A and 2G, similar to a helical structure. Furthermore,...
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